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This work was funded by Ministerio de Educación y Ciencia Project GRACCIE (CONSOLIDER-INGENIO CSD 2007-00067), CGL 2005-00642/BTE, CGL2008-05560 and CGL2006-10593, as well as Project SA008C05 and GR34 funded by Junta de Castilla y León. We are very grateful to the Integrated Ocean Drilling Program (IODP) for providing the samples for this study.